区域大气复合污染立体监测技术系统与应用

大气与环境光学学报 ›› 2009, Vol. 4 ›› Issue (4): 243-255.

区域大气复合污染立体监测技术系统与应用

刘文清刘建国谢品华陆亦怀高闽光张玉钧

中国科学院安徽光学精密机械研究所, 安徽合肥 230031

收稿日期:2009-05-28 修回日期:2009-07-09 出版日期:2009-07-28 发布日期:2009-07-24
作者简介:刘文清， (1954-) 男，江苏人，研究员、博士生导师。希腊克里特大学与欧共体克里特研究中心博士，安徽光机所环境光学与环境遥感监测技术学科带头人。毕业于中国科技大学,曾在日本国立公害研究所、意大利米兰工业大学、、日本千叶大学和德国海德堡大学做博士后、访问学者和高级访问学者。作为项目负责人多次承担国家863项目、中科院方向性创新项目、科技部科技攻关项目、省市科技攻关项目以及企业合作项目，与国外学术界有广泛的联系和学术合作。主要从事环境光学特性、有害痕量气体光学与光谱学监测方法、新型环境监测技术研究。主要已经领域为环境监测中的差分吸收光谱学（DOAS）、可调谐二极管激光光谱学（TDLAS），激光诱导荧光（LIF）、激光雷达（LIDAR）和傅里叶光谱学（FTIR）技术。
基金资助:
中国科学院知识创新工程重要方向项目“北京及周边地区奥运大气环境监测和预警联合行动计划”；北京市环境保护科技计划课题“利用光学遥感监测技术开展重要污染源区排放以及区域污染输送影响监测”

Spatio-Temporal Monitoring System and Its Application to Regional Complex Air Pollution Study

LIU Wen-qing, LIU Jian-guo, XIE Pin-hua, LU Yi-huai, GAO Min-guang, ZHANG Yu-jun

Anhui Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei 230031, China

Received:2009-05-28 Revised:2009-07-09 Published:2009-07-28 Online:2009-07-24

摘要/Abstract

摘要：

随着我国社会经济的高速发展，环境问题日益突出，各种污染物相互耦合叠加，造成我国大气污染呈现区域性、复合性以及长期性。尽管我国已建立了以城市为中心的空气质量自动监测站，但近地面有限指标的监测，不能完全反映大气污染的实际状况，使空气质量评价结果与公众直观感受不一致。也不能满足空气污染形成机制、演变和输送过程的研究需求。本文介绍了用于区域、立体、实时监测的几种技术以及利用这些技术构建的区域大气复合污染立体监测技术系统，主要用于颗粒物区域输送通量监测、气态污染物区域排放通量监测以及区域污染物垂直柱浓度监测。同时介绍了北京奥运会期间的部分监测结果，讨论了控制区域大气复合污染需要的监测技术和方法。

关键词: 区域大气, 复合污染, 立体监测

Abstract:

With the rapid economic growth of China, environmental pollution has become one of the most widely concerned issues. The air pollution in economy fast developing area has appeared regional and complex behavior by the accumulation and coupling of multi pollutants from various sources. Although many ambient air quality monitoring stations are established in urban area, the ground surface pollutant levels are limited to give the whole picture of the air pollution and reveal its real evolution process, chemical reaction scheme and regional transportation. It brings some confusion to the public by the mismatch of air quality index with the sense of atmospheric visibility. Several advanced optical and spectroscopic techniques and an integrated spatio-temporal air quality monitoring system based on them are introduced, which are applied to monitor the particulate matter regional transport flux, gaseous pollutant emission flux from area sources and distribution of vertical columns of trace gases in a large area. The partly measurement results obtained during the 2009 Beijing Olympic Games are presented. The monitoring method and techniques applied for the regional and complex air pollution study are also discussed.

Key words: regional atmosphere; complex pollution; spatio-temporal monitoring

中图分类号:

O433.4
X851

刘文清刘建国谢品华陆亦怀高闽光张玉钧. 区域大气复合污染立体监测技术系统与应用[J]. 大气与环境光学学报, 2009, 4(4): 243-255.

LIU Wen-Qing, LIU Jian-Guo, XIE Pin-Hua, LIU Yi-Huai, GAO Min-Guang, ZHANG Yu-Jun. Spatio-Temporal Monitoring System and Its Application to Regional Complex Air Pollution Study[J]. Journal of Atmospheric and Environmental Optics, 2009, 4(4): 243-255.

参考文献

[1] 周生贤. 灰霾和臭氧污染已成东部城市空气污染的突出问题 [OL]. 新华网, 2009-04-22. http://news.xinhuanet.com/newscenter/2009-04/22/content_11238371.htm.
[2] Liu Jianguo, Liu Wenqing. The current situation of environment monitoring instruments industry and the monitoring high-tech researches in China [J]. Optoelectronic Technology & Information, 2002, 15(2): 14-18(in Chinese).
刘建国, 刘文清. 我国的环境监测仪器产业状况及监测高技术创新的研究 [J]. 光电子技术与信息, 2002, 15(2): 14-18. [3] Clemitshaw K C. A review of instrumentation and measurement techniques for ground-based and airborne field studies of gas-phase tropospheric chemistry [J]. Critical Reviews in Environmental Science and Technology, 2004, 34(1): 1-108.
[4] Yang hui, Liu wenqing. Urban planetary boundary layer aerosol monitoring by Lidar at Beijng [J]. Chinese Journal Of Lasers, 2006, 33(9): 1255-1258(in Chinese).
扬辉, 刘文清. 激光雷达监测北京城区夏季边界层气溶胶 [J]. 中国激光, 2006, 33(9): 1255-1258.
[5] De Young R J, Grant W B, Severance K. Aerosol transport in the California Central Valley observed by airborne lidar [J]. Environmental Science and Technology, 2005, 39(21), 8351-8357.
[6] Chin M, Diehl T, Ginoux P, et al. Intercontinental transport of pollution and dust aerosols: implications for regional air quality [J]. Atmo. Chem. Phys., 2007, 7(21), 5501–5517.
[7] Galle B, Oppenheimer C, Geyer A, et al. A miniaturised ultraviolet spectrometer for remotesensing of SO2 fluxes: a new tool for volcano surveillance [J]. Journal of Volcanology and Geothermal Research, 2003, 119(1-4): 241-254.
[8] Li Ang, Xie Pinhua, Liu Wenqing. Monitoring of total emission from sources based on passive differential optical absorption spectroscopy [J]. Acta Optica Sinica, 2007, 27(9): 1537-1542(in Chinese).
李昂, 谢品华, 刘文清. 被动差分光学吸收光谱法监测污染源排放总量研究 [J]. 光学学报, 2007, 27(9): 1537-1542.
[9] Mellqvist J, Kihlman M, Samuelsson J, et al. The solar occultation flux (SOF) method, a new technique for the quantification of fugitive emissions of VOCs [C]. A&WMA’s 98th Annual Conference & Exhibition, Minnepolis, USA, 2005.
[10] H¨onninger G., von Friedeburg C, and Platt U. Multi axis differential optical absorption spectroscopy(MAX-DOAS) [J]. Atmos. Chem. Phys., 2004, 4: 231-254. [11] Palazzi E, Petritoli A, Ravegnani F, et al. Multiple axis DOAS measurements for the retrieval of nitrogen dioxide and ozone vertical profiles in the Presidential Estate of Castel Porziano (Rome) [C]. Proc. of SPIE, 6745: 67451Y-1.