大气与环境光学学报 ›› 2024, Vol. 19 ›› Issue (5): 589-598.

• 环境光学监测技术 • 上一篇    

2020年宣城市臭氧污染特征及气象影响因素分析

姚笛 1, 陈浩 2, 王明 2, 张帅 2*, 刘东 3   

  1. 1 宣城市生态环境局, 安徽 宣城 242099; 2 合肥中科光博量子科技有限公司, 安徽 合肥 230088; 3 中国科学院合肥物质科学研究院安徽光学精密机械研究所, 中国科学院大气光学重点实验室, 安徽 合肥 230031
  • 收稿日期:2022-07-11 修回日期:2022-11-15 出版日期:2024-09-28 发布日期:2024-10-11
  • 通讯作者: E-mail: zhangshuai@gbqtech.com E-mail:zhangshuai@gbqtech.com
  • 作者简介:姚 笛 (1987- ), 安徽庐江人, 高级工程师, 主要从事大气污染防治方面的研究。E-mail: 464830824@qq.com
  • 基金资助:
    中国科学院重点部署项目 (KFZD-SW-320), 安徽省重点研究与开发计划项目 (1804a0802196)

Characteristics of surface ozone pollution and meteorological parameters analysis in Xuancheng City in 2020

YAO Di 1, CHEN Hao 2, WANG Ming 2, ZHANG Shuai 2*, LIU Dong 3   

  1. 1 Xuancheng Ecological Environment Bureau, Xuancheng 242099, China; 2 Hefei Zhong Ke Guang Bo Quantum Science and Technology Co., Ltd., Hefei 230088, China; 3 Key Laboratory of Atmospheric Optics, Anhui Institute of Optics and Fine Mechanics, HFIPS, Chinese Academy of Sciences, Hefei 230031, China
  • Received:2022-07-11 Revised:2022-11-15 Online:2024-09-28 Published:2024-10-11
  • Contact: Shuai ZHANG E-mail:zhangshuai@gbqtech.com

摘要: 基于宣城市2020 年环境空气质量监测数据及同期气象观测数据分析了臭氧 (O3) 污染特征和气象成因。结果 表明: 2020 年臭氧日最大滑动8 小时平均质量浓度第90 百分位数 (MDA8-90) 为137 μg/m3, 相对2019 年增长了2.2%。 MDA8-90 的月变化趋势呈“M”型, 峰值出现在9 月 (164 μg/m3)。O3小时浓度日变化呈单峰型, 峰值出现在16 时, 谷值 出现在7 时。不同天气条件下, 晴天O3质量浓度峰值最高, 多云、阴天和雨天的O3浓度峰值依次递减。O3质量浓度与 气温呈现正相关性, 与相对湿度和NO2质量浓度呈现显著的负相关性。气温大于25 ℃、相对湿度小于50%及风速低于 2 m/s 的气象条件与高质量浓度O3污染密切相关。进而利用潜在源贡献函数模型分析了污染传输对宣城市O3质量浓 度的影响及潜在传输源区分布特征, 结果表明不同时期O3潜在来源差异明显, 6―8 月的主要潜在来源位于东海海面 和浙江北部区域, 而9―11 月的分布在苏皖豫鲁交界处和赣鄂交界处。

关键词: 宣城市, 臭氧, 变化特征, 气象因素, 潜在源区

Abstract: The characteristics and meteorological causes of ozone (O3) pollution in Xuancheng City, China, were analyzed based on the ambient air quality monitoring data in 2020 and the meteorological observation data of the same period. The results indicated that the 90th percentile of the maximum daily sliding 8-hour average mass concentration of O3 (MDA8-90) in 2020 was 137 μg/m3, with an increase of 2.2% compared to 2019. The monthly variation of MDA8-90 showed an "M" type, with the peak appearing in September (164 μg/m3). The diurnal variation showed a unimodal pattern, with the peak at 16:00 and the trough at 07: 00. Under different weather conditions, the peak value of O3 mass concentration was the highest on sunny days, and decreased sequentially on cloudy, overcast sky and rainy days. O3 mass concentration revealed a positive correlation with temperature and a significant negative correlation with relative humidity and NO2 concentration. Specifically, meteorological conditions with air temperatures > 25 ℃, relative humidity < 50%, and a wind speed < 2 m/s were closely related to high concentrations of O3. In addition, the potential source contribution function model (PSCF) was used to analyze the impact of pollution transport on the O3 mass concentration in Xuancheng and the distribution characteristics of potential transport sources. The results showed that the potential sources of O3 at different stages were significantly different in various periods of the year. The main potential sources of O3 from June to August were distributed in the East China Sea and the northern part of Zhejiang Province, while the main potential sources of O3 from September to November were distributed at the junction of Jiangsu, Anhui, Henan and Shandong, as well as the junction of Jiangxi and Hubei Province.

Key words: Xuancheng City, ozone, variation characteristic, meteorological factors, potential source analysis function

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