芳香化合物生成二次有机气溶胶的
光学性质研究进展

大气与环境光学学报 ›› 2022, Vol. 17 ›› Issue (1): 29-44.

• “大气气溶胶光学性质”专辑 • 上一篇下一篇

芳香化合物生成二次有机气溶胶的光学性质研究进展

李坤1∗, 王炜罡2;3, 杜林4, 葛茂发2;3

1 保罗谢尔研究所大气化学实验室, 瑞士菲利根 5232; 2 中国科学院化学研究所分子动态与稳态结构国家重点实验室, 北京 100190; 3 中国科学院大学, 北京 100049; 4 山东大学环境研究院, 山东青岛 266237

收稿日期:2021-09-13 修回日期:2021-11-27 出版日期:2022-01-28 发布日期:2022-01-28
通讯作者: E-mail: kun.li.atmos@outlook.com E-mail:kun.li.atmos@outlook.com
作者简介:李坤 (1988 - ), 山东德州人, 博士, 研究员, 主要从事二次有机气溶胶形成、成分、理化性质等方面的研究。 E-mail: kun.li.atmos@outlook.com
基金资助:
Supported by Youth Innovation Program of Universities in Shandong Province (山东省高等学校青创计划团队, 2019KJD007), National Natural Science Foundation of China (国家自然科学基金项目, 91844301, 41822703)

Optical properties of secondary organic aerosols formed from aromatic compounds: A review

LI Kun1∗, WANG Weigang2;3, DU Lin4, GE Maofa2;3

1 Laboratory of Atmospheric Chemistry, Paul Scherrer Institute, Villigen 5232, Switzerland; 2 State Key Laboratory for Structural Chemistry of Unstable and Stable Species, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China; 3 University of Chinese Academy of Sciences, Beijing 100049, China; 4 Environment Research Institute, Shandong University, Qingdao 266237, China

Received:2021-09-13 Revised:2021-11-27 Published:2022-01-28 Online:2022-01-28

摘要/Abstract

摘要： 芳香化合物是二次有机气溶胶 (SOA) 的一类重要前体物, 其在大气中的氧化可以生成具有光吸收特性的棕色碳。因此, 理解芳香化合物所生成 SOA 的光散射、光吸收、反照率等光学性质对于定量研究其对空气质量、能见度和气候变化的影响具有重要意义。系统总结了实验室研究中单环芳香烃、含氧芳香化合物、多环芳香烃三类典型芳香化合物所生成 SOA 的光学性质, 分析对比了文献关于光散射和光吸收参数的异同, 归纳了多种环境因素对 SOA 光学性质的影响, 并展望了该方向未来的重点研究领域。

关键词: 芳香化合物, 二次有机气溶胶, 棕色碳, 光散射, 光吸收

Abstract: Aromatic compounds are one important kind of precursors of secondary organic aerosol (SOA). The atmospheric oxidation of aromatic compounds can produce light-absorbing brown carbon (BrC). Therefore, understanding the optical properties (e.g., light scattering, light absorption, and single scattering albedo) of SOA formed from aromatic compounds has great implications on the quantification of their impact on air quality, visibility, and climate change. In this review, we summarise the optical properties of SOA formed from three typical kinds of aromatic compounds in laboratory studies: single-ring aromatic hydrocarbons, oxygenated aromatic compounds, and polycyclic aromatic hydrocarbons. The similarities and differences of light scattering and absorption parameters from literature are analyzed and compared, the impacts of various environmental factors on SOA optical properties are summarised, and the key research directions in the future are proposed.

Key words: aromatic compounds, secondary organic aerosol, brown carbon, light scattering, light absorption

中图分类号:

X131.1
X513

李坤∗, 王炜罡, 杜林, 葛茂发, . 芳香化合物生成二次有机气溶胶的光学性质研究进展[J]. 大气与环境光学学报, 2022, 17(1): 29-44.

LI Kun∗, WANG Weigang, DU Lin, GE Maofa, . Optical properties of secondary organic aerosols formed from aromatic compounds: A review[J]. Journal of Atmospheric and Environmental Optics, 2022, 17(1): 29-44.

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芳香化合物生成二次有机气溶胶的光学性质研究进展

Optical properties of secondary organic aerosols formed from aromatic compounds: A review

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芳香化合物生成二次有机气溶胶的 光学性质研究进展

Optical properties of secondary organic aerosols formed from aromatic compounds: A review

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芳香化合物生成二次有机气溶胶的光学性质研究进展