大气棕碳气溶胶吸光特性影响因素的研究进展

大气与环境光学学报 ›› 2022, Vol. 17 ›› Issue (1): 45-64.

• “大气气溶胶光学性质”专辑 • 上一篇下一篇

大气棕碳气溶胶吸光特性影响因素的研究进展

陈海彪1, 闫才青1;2∗, 王新锋1, 杜林1, 刘久萌3, 程远3, 郑玫4

1 山东大学环境研究院, 山东青岛 266237; 2 上海市环境科学研究院国家环境保护城市大气复合污染成因与防治重点实验室, 上海 200233; 3 哈尔滨工业大学环境学院, 黑龙江哈尔滨 150090; 4 北京大学环境科学与工程学院, 北京 100871

收稿日期:2021-09-01 修回日期:2021-10-21 出版日期:2022-01-28 发布日期:2022-01-28
通讯作者: E-mail: cyan0325@sdu.edu.cn E-mail:cyan0325@sdu.edu.cn
作者简介:陈海彪 (1997 - ), 河南开封人, 博士研究生, 主要从事棕碳气溶胶光学、理化性质方面的研究。 E-mail: haibiaoch@mail.sdu.edu.cn
基金资助:
Supported by Taishan Scholars Program of Shandong Province (山东省泰山学者青年专家计划, tsqn201909018), Qilu Youth Talent Programme of Shandong University (山东大学齐鲁青年学者计划), Youth Innovation Program of Universities in Shandong Province (山东省高等学校青创科技支持计划, 2019KJD007), State Environmental Protection Key Laboratory of Formation and Prevention of Urban Air Pollution Complex (国家环境保护城市大气复合污染成因与防治重点实验室开放基金, CX2020080585)

Research progress on light absorption properties and related influencing factors of atmospheric brown carbon aerosols

CHEN Haibiao1, YAN Caiqing1;2∗, WANG Xinfeng1, DU Lin1, LIU Jiumeng3, CHENG Yuan3, ZHENG Mei4

1 Environment Research Institute, Shandong University, Qingdao 266237, China; 2 State Environmental Protection Key Laboratory of Formation and Prevention of the Urban Air Complex, Shanghai Academy of Environmental Sciences, Shanghai 200233, China; 3 School of Environment, Harbin Institute of Technology, Harbin 150090, China; 4 College of Environmental Sciences and Engineering, Peking University, Beijing 100871, China

Received:2021-09-01 Revised:2021-10-21 Published:2022-01-28 Online:2022-01-28
Contact: Caiqing Yan E-mail:cyan0325@sdu.edu.cn

摘要/Abstract

摘要： 棕碳 (BrC) 是大气中一类重要的吸光性含碳气溶胶, 因其对区域乃至全球辐射强迫和气候具有显著影响而备受关注。然而, 对大气中 BrC 吸光特性缺乏全面认识是导致其辐射强迫评估不确定性的关键因素之一。通过梳理近年来国内外 BrC 吸光特性的相关研究, 发现 BrC 来源、发色团组成、大气过程、 pH 条件和共存金属等都是影响 BrC 吸光特性的潜在因素, 系统总结了现有研究中对 BrC 吸光特性影响因素及影响机制的认识, 并对未来 BrC 吸光特性及影响因素相关的研究方向提出了建议与展望.

关键词: 棕碳, 吸光特性, 影响因素, 研究进展, 展望

Abstract: Brown carbon (BrC) is an important class of light absorbing carbonaceous aerosols in the atmosphere, which has attracted much attention because of its significant impact on regional and even global radiative forcing and climate. However, the lack of comprehensive understanding of the optical properties of BrC in the atmosphere is one of the key factors leading to the uncertainties of its radiative forcing evaluation. Researches on light-absorbing properties of BrC at home and abroad in recent years have been reviewed. It is shown that BrC sources, chromophore composition, atmospheric process, pH conditions and coexisting metal ions are potential influencing factors of the light absorption properties of BrC. The current understanding of the influencing factors and mechanism of BrC light absorption properties are systematically summarized, and suggestions and prospects for the future research on BrC light absorption properties and associated influencing factors are also put forward.

Key words: brown carbon, light absorption properties, influencing factors, research progress, perspectives

中图分类号:

X131.1

陈海彪, 闫才青, ∗, 王新锋, 杜林, 刘久萌, 程远, 郑玫. 大气棕碳气溶胶吸光特性影响因素的研究进展[J]. 大气与环境光学学报, 2022, 17(1): 45-64.

CHEN Haibiao, YAN Caiqing, ∗, WANG Xinfeng, DU Lin, LIU Jiumeng, CHENG Yuan, ZHENG Mei. Research progress on light absorption properties and related influencing factors of atmospheric brown carbon aerosols[J]. Journal of Atmospheric and Environmental Optics, 2022, 17(1): 45-64.

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大气棕碳气溶胶吸光特性影响因素的研究进展

Research progress on light absorption properties and related influencing factors of atmospheric brown carbon aerosols

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