大气与环境光学学报 ›› 2022, Vol. 17 ›› Issue (1): 65-91.

• “大气气溶胶光学性质”专辑 • 上一篇    下一篇

基于颗粒物光学检测技术的大气沙尘气溶胶 形貌、混合态研究进展

田 雨1, 潘小乐1∗, 姚维杰1;2, 刘 航1, 张宇婷1;2, 雷山东1;2, 孙业乐1;2;3, 李 杰1, 辛金元1, 曹军骥1, 王自发1;2;3   

  1. 1 中国科学院大气物理研究所大气边界层物理与大气化学国家重点实验室, 北京 100029; 2 中国科学院大学地球与行星科学学院, 北京 100049; 3 中国科学院城市环境研究所区域大气环境研究卓越创新中心, 福建 厦门 361021
  • 收稿日期:2021-09-29 修回日期:2021-10-18 出版日期:2022-01-28 发布日期:2022-01-28
  • 通讯作者: E-mail: panxiaole@mail.iap.ac.cn E-mail:panxiaole@mail.iap.ac.cn
  • 作者简介:田 雨 (1997 - ), 女, 山东威海人, 博士, 主要从事大气沙尘气溶胶理化特性方面的研究。 E-mail: tianyu@mail.iap.ac.cn
  • 基金资助:
    Supported by Research Instrument and Equipment Development Project of Chinese Academy of Sciences (中国科学院科研仪器设备研制项 目, YJKYYQ20200009)

Research progress on atmospheric aerosol morphology and mixing state properties based on particle optical detection technology

TIAN Yu1, PAN Xiaole1∗, YAO Weijie1;2, LIU Hang1, ZHANG Yuting1;2, LEI Shandong1;2, SUN Yele1;2;3, LI Jie1, XIN Jinyuan1, CAO Junji1, WANG Zifa1;2;3   

  1. 1 State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China; 2 College of Earth and Planetary Sciences, University of Chinese Academy of Sciences, Beijing 100049, China; 3 Center of Excellence and Innovation for Regional Atmospheric Environment Research, Institute of Urban Environment, Chinese Academy of Sciences, Xiamen 361021, China
  • Received:2021-09-29 Revised:2021-10-18 Published:2022-01-28 Online:2022-01-28
  • Contact: Le XiaoPan E-mail:panxiaole@mail.iap.ac.cn

摘要: 大气中的沙尘气溶胶颗粒物会通过与太阳辐射相互作用、参与云的形成过程等, 对气候系统产生强烈影响。 对流层中的沙尘气溶胶通常是含有各种粒子成分的不均匀混合物, 只有通过详细了解单个沙尘粒子的理化特性才能 充分认识其对气候的影响效应。基于此, 对过去 20 年基于光学方法对大气沙尘气溶胶观测分析的研究进行了全面的 综述。回顾了利用电子显微镜、激光雷达以及单颗粒质谱等光学技术的研究成果, 简要介绍了基于扫描电镜和能谱、 偏光特性、非对称因子等的观测分析技术, 并讨论其优缺点; 总结了沙尘气溶胶形貌、混合态特征研究, 讨论其参与大 气物理化学过程的主要方式; 讨论了污染沙尘的光学性质、吸湿特性及成核能力, 这些特性都对气候变化和预测有重 要影响。大气中的沙尘气溶胶是复杂多样的, 如何将精确的单粒子分析技术和快速响应的在线检测技术结合将是未 来大气探测的研究重点, 这些研究成果也将进一步扩展到气溶胶的环境和气候影响研究, 以及人类健康风险评估中。

关键词: 沙尘气溶胶, 形貌特征, 混合态, 单颗粒检测, 大气化学过程, 气候效应

Abstract: Dust aerosols in the atmosphere have a strong impact on the climate system by interacting with solar radiation and participating in cloud formation. In the troposphere, dust aerosols are usually heterogeneous mixtures of various components, and their impact on climate can be fully understood only based on a detailed understanding of the physical and chemical properties of individual dust particles. The current understanding of atmospheric dust aerosols based on optical methods in the past 20 years is reviewed. The research achievements of optical techniques such as electron microscope, lidar, and single-particle mass spectrometry are summarized, the observation and analysis techniques based on scanning electron microscope and energy spectrum, polarization characteristics, and asymmetric factors are briefly introduced, and their advantages and disadvantages are discussed. The morphology and mixing state of dust aerosol are summarized, and the main ways of their participation in atmospheric physical and chemical processes are presented as well. The optical properties, hygroscopic behavior, and nucleation ability of polluted dust, all of which have important implications for climate change and prediction, are also discussed. It is well known that various aerosol particles from different sources lead to complex mixtures of dust aerosols in the atmosphere, so how to combine accurate single-particle analysis with fast response online detection technology will be the focus of future atmospheric detection research. And it is believed that these findings will be further extended to the study of the environmental and climate impacts of aerosols, as well as human health risk assessment.

Key words: dust aerosols, morphological properties, mixing state, single particle detection, atmospheric chemical process, climatic effects

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